Charge transport in organic semiconductors is notoriously extremely sensitive to the presence of disorder, both internal and external (i.e., related to interactions with the dielectric layer), especially for n-type materials. Internal dynamic disorder stems from large thermal fluctuations both in intermolecular transfer integrals and (molecular) site energies in weakly interacting van der Waals solids and sources transient localization of the charge carriers. The molecular vibrations that drive transient localization typically operate at low-frequency (

Analysis of External and Internal Disorder to Understand Band‐Like Transport in n‐Type Organic Semiconductors / Stoeckel, Marc‐antoine; Olivier, Yoann; Gobbi, Marco; Dudenko, Dmytro; Lemaur, Vincent; Zbiri, Mohamed; Guilbert, Anne A. Y.; D'Avino, Gabriele; Liscio, Fabiola; Migliori, Andrea; Ortolani, Luca; Demitri, Nicola; Jin, Xin; Jeong, Young‐gyun; Liscio, Andrea; Nardi, Marco‐vittorio; Pasquali, Luca; Razzari, Luca; Beljonne, David; Samorì, Paolo; Orgiu, Emanuele. - In: ADVANCED MATERIALS. - ISSN 0935-9648. - 33:13(2021), pp. 1-10. [10.1002/adma.202007870]

Analysis of External and Internal Disorder to Understand Band‐Like Transport in n‐Type Organic Semiconductors

Pasquali, Luca;
2021

Abstract

Charge transport in organic semiconductors is notoriously extremely sensitive to the presence of disorder, both internal and external (i.e., related to interactions with the dielectric layer), especially for n-type materials. Internal dynamic disorder stems from large thermal fluctuations both in intermolecular transfer integrals and (molecular) site energies in weakly interacting van der Waals solids and sources transient localization of the charge carriers. The molecular vibrations that drive transient localization typically operate at low-frequency (
2021
33
13
1
10
Analysis of External and Internal Disorder to Understand Band‐Like Transport in n‐Type Organic Semiconductors / Stoeckel, Marc‐antoine; Olivier, Yoann; Gobbi, Marco; Dudenko, Dmytro; Lemaur, Vincent; Zbiri, Mohamed; Guilbert, Anne A. Y.; D'Avino, Gabriele; Liscio, Fabiola; Migliori, Andrea; Ortolani, Luca; Demitri, Nicola; Jin, Xin; Jeong, Young‐gyun; Liscio, Andrea; Nardi, Marco‐vittorio; Pasquali, Luca; Razzari, Luca; Beljonne, David; Samorì, Paolo; Orgiu, Emanuele. - In: ADVANCED MATERIALS. - ISSN 0935-9648. - 33:13(2021), pp. 1-10. [10.1002/adma.202007870]
Stoeckel, Marc‐antoine; Olivier, Yoann; Gobbi, Marco; Dudenko, Dmytro; Lemaur, Vincent; Zbiri, Mohamed; Guilbert, Anne A. Y.; D'Avino, Gabriele; Lisci...espandi
File in questo prodotto:
File Dimensione Formato  
AdvMat_2021.202007870.pdf

Accesso riservato

Descrizione: Articolo principale
Tipologia: Versione pubblicata dall'editore
Dimensione 5.28 MB
Formato Adobe PDF
5.28 MB Adobe PDF   Visualizza/Apri   Richiedi una copia
2105.05202.pdf

Open access

Tipologia: Versione originale dell'autore proposta per la pubblicazione
Dimensione 5.5 MB
Formato Adobe PDF
5.5 MB Adobe PDF Visualizza/Apri
adma.202007870_accepted.pdf

Open access

Tipologia: Versione dell'autore revisionata e accettata per la pubblicazione
Dimensione 2.09 MB
Formato Adobe PDF
2.09 MB Adobe PDF Visualizza/Apri
Pubblicazioni consigliate

Licenza Creative Commons
I metadati presenti in IRIS UNIMORE sono rilasciati con licenza Creative Commons CC0 1.0 Universal, mentre i file delle pubblicazioni sono rilasciati con licenza Attribuzione 4.0 Internazionale (CC BY 4.0), salvo diversa indicazione.
In caso di violazione di copyright, contattare Supporto Iris

Utilizza questo identificativo per citare o creare un link a questo documento: https://hdl.handle.net/11380/1235816
Citazioni
  • ???jsp.display-item.citation.pmc??? 3
  • Scopus 30
  • ???jsp.display-item.citation.isi??? 27
social impact