Ultrafast 2D optical spectroscopy with 10-fs-time-resolution, complemented by density matrix simulations, show that coherent vibronic coupling accelerates polaron-pair formation and results in strongly correlated exciton and polaron-pair dynamics in polythiophene thin films at room temperature.
Coherent ultrafast polaron pair formation in a conjugated polymer at room temperature / De Sio, A., Sommer, E., Troiani, F., Rehault, J., Maiuri, M., Molinari, E., Cerullo, G., Lienau, C.. - (2016). (2016 Conference on lasers and electro-optics (CLEO) San Jose CA 05-10 June 2016).
Coherent ultrafast polaron pair formation in a conjugated polymer at room temperature
Troiani, F;Molinari, E;Cerullo, G;
2016
Abstract
Ultrafast 2D optical spectroscopy with 10-fs-time-resolution, complemented by density matrix simulations, show that coherent vibronic coupling accelerates polaron-pair formation and results in strongly correlated exciton and polaron-pair dynamics in polythiophene thin films at room temperature.
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