Deviations from the Kramers preditions resulting from the couplmg between a reactive and a non-reactwe mode arestudied in both the low- and hi&-diction Iimits. It is alsO argued how this simple picture may provide a breakdown of theupper Iimit imposed on the relaxation rate by transdion state theory.
THEORY OF ACTIVATED REACTION PROCESSES: NONLINEAR COUPLING BETWEEN REACTIVE AND NON REACTIVE MODES / M., Compiani; T., Fonseca; P., Grigolini; Serra, Roberto. - In: CHEMICAL PHYSICS LETTERS. - ISSN 0009-2614. - STAMPA. - 114:(1985), pp. 503-506.
THEORY OF ACTIVATED REACTION PROCESSES: NONLINEAR COUPLING BETWEEN REACTIVE AND NON REACTIVE MODES
SERRA, Roberto
1985
Abstract
Deviations from the Kramers preditions resulting from the couplmg between a reactive and a non-reactwe mode arestudied in both the low- and hi&-diction Iimits. It is alsO argued how this simple picture may provide a breakdown of theupper Iimit imposed on the relaxation rate by transdion state theory.
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